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The albums contain engraved portraits, autographs and correspondence of notable individuals chiefly from the United Kingdom, Belgium and France, but other countries are also represented. The vast majority of these items are from the 19th century, with an engraved portrait of the individual on the verso of the album page and a corresponding autograph/letter from that individual to Sylvain Van de Weyer or Elizabeth Van de Weyer on the recto of the album page. There is also a small grouping of older items relating to French historical figures.
Many of the items are undated, therefore the date range of the collection is taken from items which can be dated to a specific year.

This album contains documents relating to French history from the 15th to 19th centuries, portrait prints and letters relating to American history, autographs of British notables (such as William Wilberforce) and one clipping from a 17th century dutch engraving.